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dc.contributor.authorSchöbel, Jan-Hendrik
dc.contributor.authorPassia, Marco Thomas
dc.contributor.authorWolter, Nadja Anna
dc.contributor.authorPuttreddy, Rakesh
dc.contributor.authorRissanen, Kari
dc.contributor.authorBolm, Carsten
dc.date.accessioned2020-05-04T12:35:21Z
dc.date.available2020-05-04T12:35:21Z
dc.date.issued2020
dc.identifier.citationSchöbel, J.-H., Passia, M. T., Wolter, N. A., Puttreddy, R., Rissanen, K., & Bolm, C. (2020). 1,2,6-Thiadiazine 1-Oxides : Unsaturated Three-Dimensional S,N-Heterocycles from Sulfonimidamides. <i>Organic Letters</i>, <i>12</i>(7), 2702-2706. <a href="https://doi.org/10.1021/acs.orglett.0c00666" target="_blank">https://doi.org/10.1021/acs.orglett.0c00666</a>
dc.identifier.otherCONVID_34973279
dc.identifier.urihttps://jyx.jyu.fi/handle/123456789/68819
dc.description.abstractUnprecedented three-dimensional 1,2,6-thiadiazine 1-oxides have been prepared by an aza-Michael-addition/cyclization/condensation reaction sequence starting from sulfonimidamides and propargyl ketones. The products have been further functionalized by standard cross-coupling reactions, selective bromination of the heterocyclic ring, and conversion into a β-hydroxy substituted derivative. A representative product was characterized by single-crystal X-ray structure analysis.en
dc.format.mimetypeapplication/pdf
dc.languageeng
dc.language.isoeng
dc.publisherAmerican Chemical Society
dc.relation.ispartofseriesOrganic Letters
dc.rightsIn Copyright
dc.subject.othersulfonimidamides
dc.subject.othersingle-crystal X-ray
dc.title1,2,6-Thiadiazine 1-Oxides : Unsaturated Three-Dimensional S,N-Heterocycles from Sulfonimidamides
dc.typearticle
dc.identifier.urnURN:NBN:fi:jyu-202005043038
dc.contributor.laitosKemian laitosfi
dc.contributor.laitosDepartment of Chemistryen
dc.contributor.oppiaineOrgaaninen kemiafi
dc.contributor.oppiaineSoveltavan kemian yksikköfi
dc.contributor.oppiaineOrganic Chemistryen
dc.contributor.oppiaineThe Unit of Applied Chemistryen
dc.type.urihttp://purl.org/eprint/type/JournalArticle
dc.description.reviewstatuspeerReviewed
dc.format.pagerange2702-2706
dc.relation.issn1523-7060
dc.relation.numberinseries7
dc.relation.volume12
dc.type.versionacceptedVersion
dc.rights.copyright© 2020 American Chemical Society
dc.rights.accesslevelopenAccessfi
dc.relation.grantnumber298817
dc.subject.ysobioaktiiviset yhdisteet
dc.format.contentfulltext
jyx.subject.urihttp://www.yso.fi/onto/yso/p28433
dc.rights.urlhttp://rightsstatements.org/page/InC/1.0/?language=en
dc.relation.doi10.1021/acs.orglett.0c00666
dc.relation.funderSuomen Akatemiafi
dc.relation.funderAcademy of Finlanden
jyx.fundingprogramTutkijatohtori, SAfi
jyx.fundingprogramPostdoctoral Researcher, AoFen
jyx.fundinginformationWe thank the Alexander von Humboldt Foundation for support of K.R. (AvH research award), and we gratefully acknowledge Marcus Frings (RWTH Aachen University) for measuring the HPLC data. Further thanks go to Daniela Lutsch (RWTH Aachen University) for supporting practical experiments. Financial support from the Academy of Finland (RP Grant No. 298817) is also gratefully acknowledged.


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