Show simple item record

dc.contributor.authorKansanen, Kalle S. U.
dc.contributor.authorAsikainen, Aili
dc.contributor.authorToppari, J. Jussi
dc.contributor.authorGroenhof, Gerrit
dc.contributor.authorHeikkilä, Tero T.
dc.date.accessioned2020-01-16T13:33:33Z
dc.date.available2020-01-16T13:33:33Z
dc.date.issued2019
dc.identifier.citationKansanen, Kalle S. U.; Asikainen, Aili; Toppari, J. Jussi; Groenhof, Gerrit; Heikkilä, Tero T. (2019). Theory for the stationary polariton response in the presence of vibrations. Physical Review B, 100 (24), 245426. DOI: 10.1103/PhysRevB.100.245426
dc.identifier.otherCONVID_34153055
dc.identifier.urihttps://jyx.jyu.fi/handle/123456789/67341
dc.description.abstractWe construct a model describing the response of a hybrid system where the electromagnetic field—in particular, surface plasmon polaritons—couples strongly with electronic excitations of atoms or molecules. Our approach is based on the input-output theory of quantum optics, and in particular it takes into account the thermal and quantum vibrations of the molecules. The latter is described within the P(E) theory analogous to that used in the theory of dynamical Coulomb blockade. As a result, we are able to include the effect of the molecular Stokes shift on the strongly coupled response of the system. Our model then accounts for the asymmetric emission from upper and lower polariton modes. It also allows for an accurate description of the partial decoherence of the light emission from the strongly coupled system. Our results can be readily used to connect the response of the hybrid modes to the emission and fluorescence properties of the individual molecules, and thus are relevant in understanding any utilization of such systems, such as coherent light harvesting.en
dc.format.mimetypeapplication/pdf
dc.languageeng
dc.publisherAmerican Physical Society
dc.relation.ispartofseriesPhysical Review B
dc.rightsIn Copyright
dc.subject.otherplasmonics
dc.subject.otherpolaritons
dc.subject.otherhybrid quantum systems
dc.titleTheory for the stationary polariton response in the presence of vibrations
dc.typearticle
dc.identifier.urnURN:NBN:fi:jyu-202001161287
dc.contributor.laitosKemian laitosfi
dc.contributor.laitosFysiikan laitosfi
dc.contributor.laitosDepartment of Chemistryen
dc.contributor.laitosDepartment of Physicsen
dc.type.urihttp://purl.org/eprint/type/JournalArticle
dc.description.reviewstatuspeerReviewed
dc.relation.issn2469-9950
dc.relation.numberinseries24
dc.relation.volume100
dc.type.versionpublishedVersion
dc.rights.copyright© 2019 American Physical Society
dc.rights.accesslevelopenAccessfi
dc.relation.grantnumber284594 AALTO YO
dc.relation.grantnumber289947
dc.relation.grantnumber317118
dc.relation.grantnumber290677
dc.subject.ysovärähtelyt
dc.subject.ysokvanttifysiikka
dc.subject.ysopintailmiöt
dc.subject.ysokvanttikemia
dc.subject.ysoemissio (fysiikka)
dc.format.contentfulltext
jyx.subject.urihttp://www.yso.fi/onto/yso/p708
jyx.subject.urihttp://www.yso.fi/onto/yso/p5564
jyx.subject.urihttp://www.yso.fi/onto/yso/p3148
jyx.subject.urihttp://www.yso.fi/onto/yso/p19301
jyx.subject.urihttp://www.yso.fi/onto/yso/p4149
dc.rights.urlhttp://rightsstatements.org/page/InC/1.0/?language=en
dc.relation.doi10.1103/PhysRevB.100.245426
dc.relation.funderSuomen Akatemiafi
dc.relation.funderSuomen Akatemiafi
dc.relation.funderSuomen Akatemiafi
dc.relation.funderSuomen Akatemiafi
dc.relation.funderAcademy of Finlanden
dc.relation.funderAcademy of Finlanden
dc.relation.funderAcademy of Finlanden
dc.relation.funderAcademy of Finlanden
jyx.fundingprogramHuippuyksikkörahoitus, SAfi
jyx.fundingprogramAkatemiahanke, SAfi
jyx.fundingprogramAkatemiahanke, SAfi
jyx.fundingprogramAkatemiahanke, SAfi
jyx.fundingprogramCentre of Excellence, AoFen
jyx.fundingprogramAcademy Project, AoFen
jyx.fundingprogramAcademy Project, AoFen
jyx.fundingprogramAcademy Project, AoFen
jyx.fundinginformationWe acknowledge the support from the Academy of Finland Center of Excellence program (Project No. 284594) and Projects No. 289947, No. 290677, and No. 317118.


Files in this item

Thumbnail

This item appears in the following Collection(s)

Show simple item record

In Copyright
Except where otherwise noted, this item's license is described as In Copyright