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dc.contributor.authorSakaushi, Ken
dc.contributor.authorKumeda, Tomoaki
dc.contributor.authorHammes-Schiffer, Sharon
dc.contributor.authorMelander, Marko M.
dc.contributor.authorSugino, Osamu
dc.date.accessioned2020-09-07T05:06:26Z
dc.date.available2020-09-07T05:06:26Z
dc.date.issued2020
dc.identifier.citationSakaushi, K., Kumeda, T., Hammes-Schiffer, S., Melander, M. M., & Sugino, O. (2020). Advances and challenges for experiment and theory for multi-electron multi-proton transfer at electrified solid–liquid interfaces. <i>Physical Chemistry Chemical Physics</i>, <i>22</i>(35), 19401-19442. <a href="https://doi.org/10.1039/D0CP02741C" target="_blank">https://doi.org/10.1039/D0CP02741C</a>
dc.identifier.otherCONVID_41893219
dc.identifier.urihttps://jyx.jyu.fi/handle/123456789/71642
dc.description.abstractMulti-electron, multi-proton transfer is important in a wide spectrum of processes spanning biological, chemical and physical systems. These reactions have attracted significant interest due to both fundamental curiosity and potential applications in energy technology. In this Perspective Review, we shed light on modern aspects of electrode processes in the 21st century, in particular on the recent advances and challenges in multistep electron/proton transfers at solid–liquid interfaces. Ongoing developments of analytical techniques and operando spectrometry at electrode/electrolyte interfaces and reliable computational approaches to simulate complicated interfacial electrochemical reactions enable us to obtain microscopic insights about these complex processes, such as the role of quantum effects in electrochemical reactions. Our motivation in this Perspective Review is to provide a comprehensive survey and discussion of state-of-the-art developments in experiments, materials, and theories for modern electrode process science, as well as to present an outlook for the future directions in this field.en
dc.format.mimetypeapplication/pdf
dc.languageeng
dc.language.isoeng
dc.publisherRoyal Society of Chemistry (RSC)
dc.relation.ispartofseriesPhysical Chemistry Chemical Physics
dc.rightsCC BY-NC 3.0
dc.subject.othermulti-electron multi-proton transfer
dc.subject.otherelectrified solid–liquid interfaces
dc.titleAdvances and challenges for experiment and theory for multi-electron multi-proton transfer at electrified solid–liquid interfaces
dc.typearticle
dc.identifier.urnURN:NBN:fi:jyu-202009075751
dc.contributor.laitosKemian laitosfi
dc.contributor.laitosDepartment of Chemistryen
dc.contributor.oppiaineNanoscience Centerfi
dc.contributor.oppiaineNanoscience Centeren
dc.type.urihttp://purl.org/eprint/type/JournalArticle
dc.description.reviewstatuspeerReviewed
dc.format.pagerange19401-19442
dc.relation.issn1463-9076
dc.relation.numberinseries35
dc.relation.volume22
dc.type.versionpublishedVersion
dc.rights.copyright© the Owner Societies 2020
dc.rights.accesslevelopenAccessfi
dc.relation.grantnumber307853
dc.subject.ysopintakemia
dc.subject.ysosähkökemia
dc.subject.ysoelektrodit
dc.format.contentfulltext
jyx.subject.urihttp://www.yso.fi/onto/yso/p15067
jyx.subject.urihttp://www.yso.fi/onto/yso/p8093
jyx.subject.urihttp://www.yso.fi/onto/yso/p14077
dc.rights.urlhttps://creativecommons.org/licenses/by-nc/3.0/
dc.relation.doi10.1039/D0CP02741C
dc.relation.funderSuomen Akatemiafi
dc.relation.funderAcademy of Finlanden
jyx.fundingprogramTutkijatohtori, SAfi
jyx.fundingprogramPostdoctoral Researcher, AoFen
jyx.fundinginformationThis work was partially supported by JSPS KAKENHI grant numbers 19K15527 and 19H05460, and TIA collaborative research program [Kakehashi] Program No. TK19-002 and TK20-11. MMM acknowledges financial support by the Academy of Finland (project 307853) and computational resources provided by CSC – IT Services for Science.


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