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Table-top ultrafast X-ray microcalorimeter spectrometry for molecular structure

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Uhlig, J., Fullagar, W., Ullom, J., Doriese, W., Fowler, J., Swetz, D., Gador, N., Canton, S., Kinnunen, K., Maasilta, I., Bennett, C. D., Vale, L., Hilton, G., Irwin, K., Schmidt, D., & Sundström, V. (2013). Table-top ultrafast X-ray microcalorimeter spectrometry for molecular structure. Physical Review Letters, 110, Article 138302. https://doi.org/10.1103/PhysRevLett.110.138302
Published in
Physical Review Letters
Authors
Uhlig, J. |
Fullagar, W. |
Ullom, J.N. |
Doriese, W.B. |
Fowler, J.W. |
Swetz, D.S. |
Gador, N. |
Canton, S.E. |
Kinnunen, Kimmo |
Maasilta, Ilari |
Bennett, C.D.Reintsema D.A. |
Vale, L.R. |
Hilton, G.C. |
Irwin, K.D. |
Schmidt, D.R. |
Sundström, V.
Date
2013
Discipline
FysiikkaPhysics
Copyright
© 2013 American Physical Society. Published in this repository with the kind permission of the publisher.

 
This work presents an x-ray absorption measurement by use of ionizing radiation generated by a femtosecond pulsed laser source. The spectrometer was a microcalorimetric array whose pixels are capable of accurately measuring energies of individual radiation quanta. An isotropic continuum x-ray spectrum in the few-keV range was generated from a laser plasma source with a water-jet target. X rays were transmitted through a ferrocene powder sample to the detector, whose pixels have average photon energy resolution E ¼ 3:14 eV full-width-at-half-maximum at 5.9 keV. The bond distance of ferrocene was retrieved from this first hard-x-ray absorption fine-structure spectrum collected with an energydispersive detector. This technique will be broadly enabling for time-resolved observations of structural dynamics in photoactive systems.
Publisher
American Physical Society
ISSN Search the Publication Forum
0031-9007
Keywords
Experimental materials physics
DOI
https://doi.org/10.1103/PhysRevLett.110.138302
URI

http://urn.fi/URN:NBN:fi:jyu-201602011373

Publication in research information system

https://converis.jyu.fi/converis/portal/detail/Publication/23232909

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