Many-particle theory for time-dependent quantum transport in nanostructures
Julkaistu sarjassa
Research report / Department of Physics, University of JyväskyläTekijät
Päivämäärä
2012Oppiaine
FysiikkaDuring the recent decades, molecular electronics has established its place as one of the
promising fields in the nanoscience. The possibility to manufacture and control molecular
junctions where single molecules are squeezed between the conducing electrodes
has opened up new possibilities to develop nanoscale devices which could be employed
as building blocks for future nanoelectronic applications. The driving force for this new
branch of physics has been the experimental advances but also theoretical methods
have been under intensive study and many theoretical tools have been developed to
understand the electron transport processes in the nanoscale systems. This thesis focuses
on developing a formalism that helps to understand the role of electron-electron
interactions and the physical principles behind the time-dependent electron transport
in such systems.
The formalism presented in this thesis is based on the theory of non-equilibrium Green
functions (NEGF) and, more specifically on the real-time propagation of the embedded
Kadanoff-Baym (KB) equations which are quantum-kinetic equations for the oneparticle
propagator. This formalism allows for studying ultrafast dynamical processes
with femtosecond (fs) time resolution and have several advantages compared to other
methods. The Kadanoff-Baym formalism can be applied to both open and closed systems.
It allows for non-perturbative treatment of the external driving fields, suitable
preparation of the initial state, inclusion of the initial correlation effect during timepropagation
and, in addition, can deal with the electronic interactions via self-energy
terms which guarantee that the conservation laws are obeyed. All these properties are
vital for treating open and correlated systems associated to the physical phenomena
such as electron transport.
In this thesis, we apply the Kadanoff-Baym formalism to study time-dependent nonequilibrium
processes of simple correlated molecular-like systems connected to electron
reservoirs. We have found that the electron-electron interactions can have a major
impact on the time-dependent and steady-state transport properties as well as on the
spectral properties of the molecular device. The Coulomb interactions, when restricted
to the scattering region only, can lead to a significant renormalization of the molecular
gap in non-equilibrium conditions and can change the transient current flow considerably.
Furthermore, the electronic self-energies, when treated on different levels of
sophistication, can lead to very different temporal properties especially under the resonance
conditions. As one of the essential results, we have also found that the initial
correlation effects and initial state dependence, when accounted properly, can influence
considerably on the transient dynamics.
As one of the other main topics regarding the time-dependent transport, we also investigated
the role of the Coulomb interactions between the molecular scattering region and
the electron reservoirs. Our findings suggest that these interactions can have big impact
on the dynamics of the molecular junction when driven out of equilibrium with a bias voltage. We found that the Coulomb interactions between the subsystems can also lead
to strong renormalization of the resonances and change the transient and steady-state
properties dramatically. In the mean-field level, however, the treatment of these lead
interactions can give rise to current blockade and undamped post-transient dynamics
where the system does not relax towards a steady-state. These peculiar effects can be
cured with inclusion of the electron correlations which provide substantial damping to
the transients and account for the important image-charge effects via polarization diagrams.
Our results show that the lead interactions in general and the image charge
effect can modify the current–voltage characteristics prominently and that these interactions
can restrain the bias dependent quasiparticle broadening under non-equilibrium
conditions.
...
Julkaisija
University of JyväskyläISBN
978-951-39-4725-5ISSN Hae Julkaisufoorumista
0075-465XAsiasanat
aikariippuvat ilmiöt kvantti-kuljetusilmiöt elektronien kuljetusilmiöt monihiukkasteoria Greenin funktio itseisenergia Kadanoff-Baym time-dependent non-equilibrium phenomena quantum transport electron transport many-particle theory Green function self-energy fysiikka molekyylielektroniikka elektronit
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