Theory for polaritonic quantum tunneling
Kansanen, K. S. U. (2023). Theory for polaritonic quantum tunneling. Physical Review B, 107(3), Article 035405. https://doi.org/10.1103/PhysRevB.107.035405
Julkaistu sarjassa
Physical Review BTekijät
Päivämäärä
2023Tekijänoikeudet
© 2023 American Physical Society
I investigate the tunneling decay rate of a polaritonic system formed by a strong coupling between a vacuum cavity mode and N metastable systems. Using a simple model potential, I find the instanton solutions controlling the low-temperature tunneling rate. The resulting rate modification due to the cavity is proportional to the mean of the second power of the light-matter coupling. No collective effect that would enhance the rates by a factor of √N is present, which is in line with the results in the thermal activation regime.
Julkaisija
American Physical Society (APS)ISSN Hae Julkaisufoorumista
2469-9950Asiasanat
Julkaisu tutkimustietojärjestelmässä
https://converis.jyu.fi/converis/portal/detail/Publication/176902404
Metadata
Näytä kaikki kuvailutiedotKokoelmat
Rahoittaja(t)
Suomen AkatemiaRahoitusohjelmat(t)
Akatemiahanke, SALisätietoja rahoituksesta
This work has been supported by the Magnus Ehrnrooth foundation and the Academy of Finland (Projects No. 317118 and No. 321982).Lisenssi
Samankaltainen aineisto
Näytetään aineistoja, joilla on samankaltainen nimeke tai asiasanat.
-
Multi-scale dynamics simulations of molecular polaritons : the effect of multiple cavity modes on polariton relaxation
Tichauer, Ruth H.; Feist, Johannes; Groenhof, Gerrit (AIP Publishing, 2021)Coupling molecules to the confined light modes of an optical cavity is showing great promise for manipulating chemical reactions. However, to fully exploit this principle and use cavities as a new tool for controlling ... -
Photochemical initiation of polariton-mediated exciton propagation
Sokolovskii, Ilia; Groenhof, Gerrit (De Gruyter, 2024)Placing a material inside an optical cavity can enhance transport of excitation energy by hybridizing excitons with confined light modes into polaritons, which have a dispersion that provides these light–matter quasi-particles ... -
Polariton-assisted long-distance energy transfer between excitons in two-dimensional semiconductors
Pajunpää, Tuomas; Nigmatulin, Fedor; Akkanen, Suvi-Tuuli; Fernandez, Henry; Groenhof, Gerrit; Sun, Zhipei (American Physical Society (APS), 2024)Strong exciton-photon coupling offers an effective path for polariton-mediated long-distance coherent energy transfer (ET) between excitonic states. Here, we demonstrate strong coupling between excitons in WS2 monolayers, ... -
Polariton response in the presence of Brownian dissipation from molecular vibrations
Kansanen, Kalle S. U.; Toppari, J. Jussi; Heikkilä, Tero T. (American Institute of Physics, 2021)We study the elastic response of a stationarily driven system of a cavity field strongly coupled with molecular excitons, taking into account the main dissipation channels due to the finite cavity linewidth and molecular ... -
Theory for the stationary polariton response in the presence of vibrations
Kansanen, Kalle S. U.; Asikainen, Aili; Toppari, J. Jussi; Groenhof, Gerrit; Heikkilä, Tero T. (American Physical Society, 2019)We construct a model describing the response of a hybrid system where the electromagnetic field—in particular, surface plasmon polaritons—couples strongly with electronic excitations of atoms or molecules. Our approach is ...
Ellei toisin mainittu, julkisesti saatavilla olevia JYX-metatietoja (poislukien tiivistelmät) saa vapaasti uudelleenkäyttää CC0-lisenssillä.