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dc.contributor.authorLindgren, Johan
dc.contributor.authorHulkko, Eero
dc.contributor.authorPettersson, Mika
dc.contributor.authorKiljunen, Toni
dc.date.accessioned2012-01-23T09:10:04Z
dc.date.available2012-01-23T09:10:04Z
dc.date.issued2011
dc.identifier.citationLindgren, J., Hulkko, E., Pettersson, M., & Kiljunen, T. (2011). Rotational coherence imaging and control for CN molecules through time-frequency resolved coherent anti-Stokes Raman scattering. <i>The Journal of Chemical Physics</i>, <i>135</i>(22), 224514-8. <a href="https://doi.org/10.1063/1.3665934" target="_blank">https://doi.org/10.1063/1.3665934</a>
dc.identifier.otherCONVID_21002012
dc.identifier.otherTUTKAID_49025
dc.identifier.urihttps://jyx.jyu.fi/handle/123456789/37231
dc.description.abstractNumerical wave packet simulations are performed for studying coherent anti-Stokes Raman scattering (CARS) for CN radicals. Electronic coherence is created by femtosecond laser pulses between the X²Σ and B²Σ states. Due to the large energy separation of vibrational states, the wave packets are superpositions of rotational states only. This allows for a specially detailed inspection of the second- and third-order coherences by a two-dimensional imaging approach. We present the time-frequency domain images to illustrate the intra- and intermolecular interferences, and discuss the procedure to rationally control and experimentally detect the interferograms in solid Xe environment.fi
dc.language.isoeng
dc.publisherAmerical Institute of Physics
dc.relation.ispartofseriesThe Journal of Chemical Physics
dc.subject.otherkoherentti anti-Stokes Raman spektroskopia
dc.subject.otherhiiliyhdisteet
dc.subject.otherrotaatiotilat
dc.subject.othervibraatiotilat
dc.subject.othercoherent antiStokes Raman scattering
dc.subject.othercarbon combounds
dc.subject.otherrotationla states
dc.subject.othervibrational states
dc.titleRotational coherence imaging and control for CN molecules through time-frequency resolved coherent anti-Stokes Raman scattering
dc.typearticle
dc.identifier.urnURN:NBN:fi:jyu-201201211051
dc.contributor.laitosKemian laitosfi
dc.contributor.laitosDepartment of Chemistryen
dc.contributor.oppiaineFysikaalinen kemiafi
dc.contributor.oppiaineNanoscience Centerfi
dc.contributor.oppiainePhysical Chemistryen
dc.contributor.oppiaineNanoscience Centeren
dc.type.urihttp://purl.org/eprint/type/JournalArticle
dc.date.updated2012-01-21T04:30:04Z
dc.type.coarhttp://purl.org/coar/resource_type/c_2df8fbb1
dc.description.reviewstatuspeerReviewed
dc.format.pagerange224514-8
dc.relation.issn0021-9606
dc.relation.numberinseries22
dc.relation.volume135
dc.type.versionpublishedVersion
dc.rights.copyright© 2011 American Institute of Physics
dc.rights.accesslevelopenAccessfi
dc.subject.ysovapaat radikaalit
dc.subject.ysonumeerinen analyysi
jyx.subject.urihttp://www.yso.fi/onto/yso/p2983
jyx.subject.urihttp://www.yso.fi/onto/yso/p15833
dc.relation.doi10.1063/1.3665934
dc.type.okmA1


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